DanskDTU.dkIndexContactPhone bookDTU AlumniPortalen
Title: Site Specificity in Femtosecond Laser Desorption of Neutral H Atoms from Graphite(0001)
Type: Journal articleJournal article
Participant(s):
Forfatter:  Frigge, R.
Technical University of Denmark

Forfatter:  Hoger, T.
Technical University of Denmark

Forfatter:  Siemer, B.
Technical University of Denmark

Forfatter:  Witte, H.
Technical University of Denmark

Forfatter:  Silies, M.
Technical University of Denmark

Forfatter:  Zacharias, H
Technical University of Denmark

Author:  Olsen, Thomas (Cwisno: 40609)
Technical University of Denmark
Email:

Author:  Schiøtz, Jakob (Cwisno: 2737)
Technical University of Denmark
Email:

Abstract: Femtosecond laser excitation and density functional theory reveal site and vibrational state specificity in neutral atomic hydrogen desorption from graphite induced by multiple electronic transitions. Multimodal velocity distributions witness the participation of ortho and para pair states of chemisorbed hydrogen in the desorption process. Very slow velocities of 700 and 400  ms-1 for H and D atoms are associated with the desorption out of the highest vibrational state of a barrierless potential.
Published: in journal: Physical Review Letters (ISSN: 0031-9007) (DOI: http://dx.doi.org/10.1103/PhysRevLett.104.256102), vol: 104, issue: 25, pages: 256102, 2010
DOI:
File(s):
See the publication in DTU Orbit See the publication in DTU Orbit

Top
FysikvejBuilding 3112800 Kgs. LyngbyTel +45 4525 3344VAT 30060946EAN 5798000431010/5798000431027
Cookies